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Not sure where you are coming up with your numbers. Here is the label for a popular 2,4-D Herbicide:
Goatheads are easy to kill but they are persistent little bastards so the drop-dead concentration of the above is a 0.75% Spray Concentration or 0.3 cups / gallon of water. If they already have yellow flowers, you are way too late and that crop is in the ground and you will be dealing with it next year.
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Yellow flowers are a sign of post emergent activity, and are an indication of the plant beginning the seed cycle.
Once it has the green seeds on there....your gonna need to manually pull the plant to prevent the seeds from getting into the soil.
Whats amazing about the plant...if the green seeds are present, and you spray it....the plant will use the last bit of life to mature the seeds to viability.
Lot's of folks buy their stuff at HD or Lowes, and may not read the labels for concentration levels.
2,4-D levels in many of the brand-name pre-mixed or ready to use products are generally much lower like, 10-15%.....so as a baseline, I recommend using a product with at least 15% or better for effectiveness.
My go-to is the Amine 400 concentrate on goat heads, and hard-to-kill weeds and brush, in a mix with glyphosate, as TSC usually has it in stock.
But the biggest take-away here is .....don't be complacent !!
Get out there and pull what you can, spray what you can, and make the effort to eradicate these bastards !!