On the subject of grease as an AR lubricant in general, in my opinion grease is far superior to oil. It lasts much longer, works as a sealant to keep out contamination and stays where you put it. I use grease exclusively on my ARs (Super Lube NLGI 2).
That being said, not all grease is suitable for firearms lubrication. Specifically, Aeroshell 33ms/64 is a lithium complex grease - which is a good choice for a thickener - but its operating temp range seems a bit low. For example, Aeroshell 33ms/64 has an operating temp range of -99 to 250f, whereas Super Lube is -45 to 450f. I'm not a grease expert or anything, so maybe it'd be fine, but I'd be looking for something with a bit wider operating temp range for an AR lubricant. Basically, if it doesn't run off too badly when the weapon starts getting hot, and it isn't too thick for your average temps, then it should work.